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Magnetite impregnation effects on the sorbent properties of activated carbons and biochars

Titelangaben

Han, Zhantao ; Sani, Badruddeen ; Mrozik, Wojciech ; Obst, Martin ; Beckingham, Barbara ; Karapanagioti, Hrissi K. ; Werner, David:
Magnetite impregnation effects on the sorbent properties of activated carbons and biochars.
In: Water Research. Bd. 70 (2015) . - S. 394-403.
DOI: https://doi.org/10.1016/j.watres.2014.12.016

Abstract

This paper discusses the sorbent properties of magnetic activated carbons and biochars produced by wet impregnation with iron oxides. The sorbents had magnetic susceptibil- ities consistent with theoretical predictions for carbon-magnetite composites. The high BET surface areas of the activated carbons were preserved in the synthesis, and enhanced for one low surface area biochar by dissolving carbonates. Magnetization decreased the point of zero charge. Organic compound sorption correlated strongly with BET surface areas for the pristine and magnetized materials, while metal cation sorption did not show such a correlation. Strong sorption of the hydrophobic organic contaminant phenanthrene to the activated carbon or biochar surfaces was maintained following magnetite impreg- nation, while phenol sorption was diminished, probably due to enhanced carbon oxidation. Copper, zinc and lead sorption to the activated carbons and biochars was unchanged or slightly enhanced by the magnetization, and iron oxides also contributed to the composite metal sorption capacity. While a magnetic biochar with 219 ± 3.7 m2/g surface area nearly reached the very strong organic pollutant binding capacity of the two magnetic activated carbons, a magnetic biochar with 68 ± 2.8 m2/g surface area was the best metal sorbent. Magnetic biochars thus hold promise as more sustainable alternatives to coal-derived magnetic activated carbons.

Weitere Angaben

Publikationsform: Artikel in einer Zeitschrift
Begutachteter Beitrag: Ja
Zusätzliche Informationen: BAYCEER135367
Institutionen der Universität: Forschungseinrichtungen
Forschungseinrichtungen > Forschungszentren
Forschungseinrichtungen > Forschungszentren > Bayreuther Zentrum für Ökologie und Umweltforschung - BayCEER
Titel an der UBT entstanden: Ja
Themengebiete aus DDC: 500 Naturwissenschaften und Mathematik
Eingestellt am: 29 Jul 2016 07:07
Letzte Änderung: 29 Jul 2016 07:07
URI: https://eref.uni-bayreuth.de/id/eprint/33688