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Toward Far-field Vibrational Spectroscopy of Single Molecules at Room Temperature

Title data

Winterhalder, M. J. ; Zumbusch, A. ; Lippitz, Markus ; Orrit, Michel:
Toward Far-field Vibrational Spectroscopy of Single Molecules at Room Temperature.
In: The Journal of Physical Chemistry B. Vol. 115 (May 2011) Issue 18 . - pp. 5425-5430.
ISSN 1520-5207
DOI: https://doi.org/10.1021/jp109652s

Abstract in another language

We propose a new scheme for the extraction of chemically sensitive vibrational information from a single fluorescent molecule at room temperature. Our approach is based on a three-photon fluorescence excitation scheme, with selectivity in the production of a vibrational population of the ground state. We estimate the expected signal in perturbation theory for a standard dye molecule, compare its magnitude qualitatively to noise and various background sources, and discuss the experimental realization of this scheme.

Further data

Item Type: Article in a journal
Refereed: Yes
Institutions of the University: Faculties
Faculties > Faculty of Mathematics, Physics und Computer Science
Faculties > Faculty of Mathematics, Physics und Computer Science > Department of Physics
Faculties > Faculty of Mathematics, Physics und Computer Science > Department of Physics > Lehrstuhl Experimentalphysik III - Nanooptik
Faculties > Faculty of Mathematics, Physics und Computer Science > Department of Physics > Lehrstuhl Experimentalphysik III - Nanooptik > Lehrstuhl Experimentalphysik III - Nanooptik - Univ.-Prof. Dr. Markus Lippitz
Result of work at the UBT: No
DDC Subjects: 500 Science
500 Science > 500 Natural sciences
500 Science > 530 Physics
Date Deposited: 16 Dec 2015 08:26
Last Modified: 10 Apr 2018 09:02
URI: https://eref.uni-bayreuth.de/id/eprint/28957