Title data
Metzger, Bernd ; Schumacher, Thorsten ; Hentschel, Mario ; Lippitz, Markus ; Giessen, Harald:
Third Harmonic Mechanism in Complex Plasmonic Fano Structures.
In: ACS Photonics.
Vol. 1
(2014)
Issue 6
.
- pp. 471-476.
ISSN 2330-4022
DOI: https://doi.org/10.1021/ph5000677
Abstract in another language
We perform third harmonic spectroscopy of dolmen-type nanostructures, which exhibit plasmonic Fano resonances in the near-infrared. Strong third harmonic emission is predominantly radiated close to the low energy peak of the Fano resonance. Furthermore, we find that the third harmonic polarization of the subradiant mode interferes destructively and diminishes the nonlinear signal in the far-field. By comparing the experimental third harmonic spectra with finite element simulations and an anharmonic oscillator model, we find strong indications that the source of the third harmonic is the optical nonlinearity of the bare gold enhanced by the resonant plasmonic polarization.
Further data
Item Type: | Article in a journal |
---|---|
Refereed: | Yes |
Institutions of the University: | Faculties > Faculty of Mathematics, Physics und Computer Science > Department of Physics > Chair Experimental Physics III - Nanooptics > Chair Experimental Physics III - Nanooptics - Univ.-Prof. Dr. Markus Lippitz Faculties Faculties > Faculty of Mathematics, Physics und Computer Science Faculties > Faculty of Mathematics, Physics und Computer Science > Department of Physics Faculties > Faculty of Mathematics, Physics und Computer Science > Department of Physics > Chair Experimental Physics III - Nanooptics |
Result of work at the UBT: | Yes |
DDC Subjects: | 500 Science > 530 Physics |
Date Deposited: | 13 Nov 2015 13:36 |
Last Modified: | 24 Jan 2022 14:36 |
URI: | https://eref.uni-bayreuth.de/id/eprint/22209 |