Title data
Winterhalder, M. J. ; Zumbusch, A. ; Lippitz, Markus ; Orrit, Michel:
Toward Far-field Vibrational Spectroscopy of Single Molecules at Room Temperature.
In: The Journal of Physical Chemistry B.
Vol. 115
(2011)
Issue 18
.
- pp. 5425-5430.
ISSN 1520-5207
DOI: https://doi.org/10.1021/jp109652s
Abstract in another language
We propose a new scheme for the extraction of chemically sensitive vibrational information from a single fluorescent molecule at room temperature. Our approach is based on a three-photon fluorescence excitation scheme, with selectivity in the production of a vibrational population of the ground state. We estimate the expected signal in perturbation theory for a standard dye molecule, compare its magnitude qualitatively to noise and various background sources, and discuss the experimental realization of this scheme.
Further data
Item Type: | Article in a journal |
---|---|
Refereed: | Yes |
Institutions of the University: | Faculties Faculties > Faculty of Mathematics, Physics und Computer Science Faculties > Faculty of Mathematics, Physics und Computer Science > Department of Physics Faculties > Faculty of Mathematics, Physics und Computer Science > Department of Physics > Chair Experimental Physics III - Nanooptics Faculties > Faculty of Mathematics, Physics und Computer Science > Department of Physics > Chair Experimental Physics III - Nanooptics > Chair Experimental Physics III - Nanooptics - Univ.-Prof. Dr. Markus Lippitz |
Result of work at the UBT: | No |
DDC Subjects: | 500 Science 500 Science > 500 Natural sciences 500 Science > 530 Physics |
Date Deposited: | 16 Dec 2015 08:26 |
Last Modified: | 24 Jan 2022 14:48 |
URI: | https://eref.uni-bayreuth.de/id/eprint/28957 |