Title data
Unterkofler, Sarah ; Pflock, Tobias ; Southall, June ; Cogdell, Richard J. ; Köhler, Jürgen:
Fluorescence blinking of the RC-LH1 complex from Rhodopseudomonas palustris.
In: ChemPhysChem.
Vol. 12
(2011)
Issue 3
.
- pp. 711-716.
ISSN 1439-4235
DOI: https://doi.org/10.1002/cphc.201000588
Abstract in another language
We investigate fluorescence blinking of individual RC-LH1 (reaction-centre-light-harvesting 1) complexes from the photosynthetic purple bacterium Rhodopseudomonas palustris. For both the on- and off-periods the telegraph-like intermittency of the fluorescence intensity follows power-law statistics with exponents between 1 and 2. Yet, this behaviour was only observed for a small fraction of the complexes studied. We argue that the majority of the complexes reside in a prolonged on-state, due to a mechanism that is similar to the Coulomb blockade in semiconductor quantum dots, and which results here from the photoinduced charges located within the RC upon photoexcitation of the LH1 antenna.
Further data
Item Type: | Article in a journal |
---|---|
Refereed: | Yes |
Keywords: | spectroscopic methods |
Institutions of the University: | Faculties > Faculty of Mathematics, Physics und Computer Science > Department of Physics > Chair Experimental Physics IX - Spectroscopy of Soft Matter > Chair Experimental Physics IX - Spectroscopy of Soft Matter - Univ.-Prof. Dr. Jürgen Köhler Faculties Faculties > Faculty of Mathematics, Physics und Computer Science Faculties > Faculty of Mathematics, Physics und Computer Science > Department of Physics Faculties > Faculty of Mathematics, Physics und Computer Science > Department of Physics > Chair Experimental Physics IX - Spectroscopy of Soft Matter |
Result of work at the UBT: | Yes |
DDC Subjects: | 500 Science > 530 Physics |
Date Deposited: | 12 Apr 2018 13:22 |
Last Modified: | 11 Jan 2023 11:00 |
URI: | https://eref.uni-bayreuth.de/id/eprint/43408 |