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Chee, See Wee ; Lunkenbein, Thomas ; Schlögl, Robert ; Roldán Cuenya, Beatriz:
Operando Electron Microscopy of Catalysts: The Missing Cornerstone in Heterogeneous Catalysis Research?
In: Chemical Reviews.
Bd. 123
(2023)
Heft 23
.
- S. 13374-13418.
ISSN 0009-2665
DOI: https://doi.org/10.1021/acs.chemrev.3c00352
Abstract
Heterogeneous catalysis in thermal gas-phase and electrochemical liquid-phase chemical conversion plays an important role in our modern energy landscape. However, many of the structural features that drive efficient chemical energy conversion are still unknown. These features are, in general, highly distinct on the local scale and lack translational symmetry, and thus, they are difficult to capture without the required spatial and temporal resolution. Correlating these structures to their function will, conversely, allow us to disentangle irrelevant and relevant features, explore the entanglement of different local structures, and provide us with the necessary understanding to tailor novel catalyst systems with improved productivity. This critical review provides a summary of the still immature field of operando electron microscopy for thermal gas-phase and electrochemical liquid-phase reactions. It focuses on the complexity of investigating catalytic reactions and catalysts, progress in the field, and analysis. The forthcoming advances are discussed in view of correlative techniques, artificial intelligence in analysis, and novel reactor designs.
Weitere Angaben
| Publikationsform: | Artikel in einer Zeitschrift |
|---|---|
| Begutachteter Beitrag: | Ja |
| Zusätzliche Informationen: | WOS:001125353100001 |
| Institutionen der Universität: | Fakultäten > Fakultät für Biologie, Chemie und Geowissenschaften > Fachgruppe Chemie |
| Titel an der UBT entstanden: | Nein |
| Themengebiete aus DDC: | 500 Naturwissenschaften und Mathematik > 540 Chemie |
| Eingestellt am: | 12 Jun 2025 08:23 |
| Letzte Änderung: | 12 Jun 2025 08:23 |
| URI: | https://eref.uni-bayreuth.de/id/eprint/93667 |