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Wolff, Veronika ; Trebs, Ivonne ; Foken, Thomas ; Meixner, Franz X.:
Exchange of reactive nitrogen compounds : concentrations and fluxes of total ammonium and total nitrate above a spruce forest canopy.
In: Biogeosciences Discussions.
Bd. 6
(2009)
.
- S. 10663-10706.
ISSN 1810-6285
DOI: https://doi.org/10.5194/bgd-6-10663-2009
Abstract
Total ammonium (tot-NH4+) and total nitrate (tot-NO3−) provide a chemically conservative quantity in the measurement of exchange processes of reactive nitrogen compounds ammonia (NH3), particulate ammonium (NH4+), nitric acid (HNO3), and particulate nitrate (NO3−), using the aerodynamic gradient method. Total fluxes were derived from concentration differences of total ammonium (NH3 and NH4+) and total nitrate (HNO3 and NO3−) measured at two levels. Gaseous species and related particulate compounds were measured selectively, simultaneously and continuously above a spruce forest canopy in south-eastern Germany in summer 2007. Measurements were performed using a wet-chemical two-point gradient instrument, the GRAEGOR. Median concentrations of NH3, HNO3, NH4−, and NO3− were 0.57, 0.12, 0.76, and 0.48 μg m−3, respectively. Total ammonium and total nitrate fluxes showed large variations depending on meteorological conditions, with concentrations close to zero under humid and cool conditions and higher concentrations under dry conditions. Mean fluxes of total ammonium and total nitrate in September 2007 were directed towards the forest canopy and were −65.77 ng m−2 s−1 and −41.02 ng m−2 s−1 (in terms of nitrogen), respectively. Their deposition was controlled by aerodynamic resistances only, with very little influence of surface resistances. Including measurements of wet deposition and findings of former studies at the study site on occult deposition (fog water interception), the total N deposition in September 2007 was estimated to 5.86 kg ha−1.
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| Publikationsform: | Artikel in einer Zeitschrift |
|---|---|
| Begutachteter Beitrag: | Ja |
| Zusätzliche Informationen: | BAYCEER76435 |
| Institutionen der Universität: | Fakultäten > Fakultät für Biologie, Chemie und Geowissenschaften > Fachgruppe Geowissenschaften > Ehemalige Professoren > Professur Mikrometeorologie - Univ.-Prof. Dr. Thomas Foken Forschungseinrichtungen > Forschungszentren > Bayreuther Zentrum für Ökologie und Umweltforschung - BayCEER Fakultäten Fakultäten > Fakultät für Biologie, Chemie und Geowissenschaften Fakultäten > Fakultät für Biologie, Chemie und Geowissenschaften > Fachgruppe Geowissenschaften Fakultäten > Fakultät für Biologie, Chemie und Geowissenschaften > Fachgruppe Geowissenschaften > Ehemalige Professoren Forschungseinrichtungen Forschungseinrichtungen > Forschungszentren |
| Titel an der UBT entstanden: | Ja |
| Themengebiete aus DDC: | 500 Naturwissenschaften und Mathematik |
| Eingestellt am: | 21 Aug 2015 06:49 |
| Letzte Änderung: | 21 Apr 2022 13:26 |
| URI: | https://eref.uni-bayreuth.de/id/eprint/18431 |