Dressed-state analysis of two-color excitation schemes

Titelangaben

Bracht, Thomas K. ; Seidelmann, Tim ; Karli, Yusuf ; Kappe, Florian ; Remesh, Vikas ; Weihs, Gregor ; Axt, Vollrath Martin ; Reiter, Doris E.:
Dressed-state analysis of two-color excitation schemes.
In: Physical Review B. Bd. 107 (2023) Heft 3 . - 035425.
ISSN 0163-1829
DOI: https://doi.org/10.1103/PhysRevB.107.035425

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Abstract

To coherently control a few-level quantum emitter, typically pulses with an energy resonant to the transition energy are applied, making use of the Rabi mechanism, while a single off-resonant pulse does not result in a population inversion. Surprisingly, a two-color excitation with a combination of two off-resonant pulses is able to invert the system. In this paper, we provide an in-depth analysis of two-color excitation schemes within the dressed-state picture. We show that such schemes can be understood as a driving of the transition between the dressed states. In the two-level system this allows us to derive analytic expressions for the pulse parameters yielding a population inversion. We relate our findings to the Swing-UP of quantum EmitteR population (SUPER) mechanism, where the two pulses are red detuned. Our interpretation also holds in the case where one pulse is red detuned while the other pulse is blue detuned, as in dichromatic excitation schemes. We extend our considerations of the SUPER mechanism to the three-level system, where a strong mixing between the bare states takes place. The insights gained from these results help in finding accessible regimes for further experimental realizations of two-color excitation schemes.